Journal
JOURNAL OF MEMBRANE SCIENCE
Volume 637, Issue -, Pages -Publisher
ELSEVIER
DOI: 10.1016/j.memsci.2021.119627
Keywords
MXene membrane; Super-hydrophilicity/underwater super-oleophobicity; beta-FeOOH; Self-cleaning; Oil/water separation
Categories
Funding
- National Natural Science Foundation of China [51903215]
- Sichuan Province SciTech Supported Project [2020YJ0168]
- International Science and Technology Cooperation Project from Chengdu Municipal Government [2020GH0200074HZ]
- Sichuan Youth Science and Technology Innovation Research Team Project [2020JDTD0018]
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This study presents a facile strategy to fabricate a two-dimensional MXene-based composite membrane with excellent permeation flux and separation efficiency, along with outstanding anti-fouling resistance and durability, even in harsh conditions, maintaining highly efficient oil/water separation performance.
Super-wetting membranes with outstanding permeation and anti-fouling performance are promising candidates for highly-efficient oily wastewater treatment. Herein, we designed a facile strategy to fabricate the superhydrophilic/underwater super-oleophobic two-dimensional MXene-based composite membrane via vacuum assisted self-assembly of two-dimensional MXene nanosheets on porous polyvinylidene fluoride (PVDF) substrate and in situ mineralization of photocatalyst beta-FeOOH on the membrane surface. Benefiting from the inherent super-wettability and regulated lamellar structure (Short transport pathway and abundant nano channels), the resultant MXene-based composite membrane displayed fast permeation flux (500.38-1022.7 L m(-2) h(-1)) and favorable separation efficiency (99.32-99.72%) for a series of micro-scaled oil-in-water emulsions. Importantly, the excellent photo-induced self-cleaning capability and low oil-adhesion contributed to the high anti-fouling resistance, outstanding reusability, and durability of 2D MXene composite membrane. Moreover, the 2D MXene composite membrane exhibited superior chemical stability, which enabled it to maintain highly efficient oil/water separation performance in high-temperature, high salty, and strongly corrosive conditions. This work provides a feasible route to fabricate durable super-wetting 2D membranes with photo-Fenton selfcleaning capability for the oily wastewater treatment in harsh environments.
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