4.2 Article

Bi/BiVO4/NiFe-LDH heterostructures with enhanced photoelectrochemical performance for streptomycin detection

Journal

JOURNAL OF ENVIRONMENTAL SCIENCES
Volume 109, Issue -, Pages 114-122

Publisher

SCIENCE PRESS
DOI: 10.1016/j.jes.2021.03.043

Keywords

Detection; Heterojunction; Photoelectrochemical sensor; Streptomycin

Funding

  1. Key projects of science and technology research in Hebei Higher Education Institutions [ZD2018311, ZD2020417]
  2. Local science and technology development fund projects [206Z1402G]
  3. Science and Technology Research Project of Colleges and Universities in Hebei Province [BJ2019203]
  4. Xingtai Science and Technology Program [2018ZC031, 2018ZC227, 2019ZZ023, 2019ZX07]

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The study developed a novel PEC sensor for detecting streptomycin, which demonstrated ultra-high sensitivity and selectivity. The Bi/BiVO4/LDH heterostructures prepared in this work showed good photoactivity in the visible light range, enhancing the material's photocurrent response.
Streptomycin (STR) plays an essential role in bacterial infection treatments. Selectivity and sensitivity of photoelectrochemical (PEC) sensors are the two most important parameters, which can be measured using the photosensitivity of its active material. We prepared a novel PEC sensor to detect STR using Bi/BiVO 4 /LDH (layered double hydroxides) heterostructures as an active material, which is photoactive in the visible light wavelength range. The simultaneous presence of LDH and Bi/BiVO 4 enhanced the material photocurrent response, which was linear to the STR concentrations in the 0.01-500 nmol/L range. The STR detection limit by this sensor was 0.0042 nmol/L. Our novel PEC-based sensing strategy includes using an ultra-sensitive and highly selective sensor for STR detection. Additionally, the two-pot synthesis of Bi/BiVO 4 /LDH developed in this work is environmentally friendly. (c) 2021 The Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences. Published by Elsevier B.V.

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