4.7 Article

A generalizable strategy for constructing ultralight three-dimensional hierarchical network heterostructure as high-efficient microwave absorber

Journal

JOURNAL OF COLLOID AND INTERFACE SCIENCE
Volume 605, Issue -, Pages 13-22

Publisher

ACADEMIC PRESS INC ELSEVIER SCIENCE
DOI: 10.1016/j.jcis.2021.07.054

Keywords

Three-dimensional interconnected network; Reduced graphene oxide foam/MoS2 nanosheets; Strong absorption capability; Broad frequency bandwidth; Thin matching thicknesses

Funding

  1. Fund of Fok Ying Tung Education Foundation
  2. Guizhou Province Graduate Research Fund [2020-089]
  3. Major Research Project of innovative Group of Guizhou province [2018-013]
  4. National Science Foundation of China [11964006, 11774156]
  5. Foundation of the National Key Project for Basic Research [2012CB932304]

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The study focuses on designing and fabricating high-efficient microwave absorbers using graphene oxide foam and reduced graphene oxide foam/MoS2 nanosheets. These samples exhibit ultralow density, excellent microwave absorption properties, and are ideal for improving MAs performance.
Using previous models and theories to construct and develop high-efficient microwave absorbers (MAs) should be a strategic and effective ways to optimize the electromagnetic wave attenuation. Herein, the ultralow density and flexible graphene oxide foam (GOF) and reduced graphene oxide foam (RGOF)/MoS2 nanosheets were designed and fabricated by the method of chemical vapor deposition and hydrothermal reaction. The obtained GOF and RGOF/MoS2 samples exhibited very excellent microwave absorption properties while their densities were merely 0.0082 and 0.0084 g.cm(3), respectively. More importantly, benefiting from the excellent synergistic effect between RGOF and MoS2, the designed RGOF/MoS2 well inherited the combined advantages of GOF and MoS2 in terms of strong absorption abilities, broad absorption bandwidth and thin matching thicknesses. The values of minimum reflection loss and effective frequency bandwidth for RGOF/MoS2 sample could reach up to -62.92 dB with the matching thickness of 2.27 mm and 4.48 GHz with the matching thickness of 2.12 mm, which were very desirable for high-performance MAs. Moreover, the obtained results indicated that the microwave absorption properties of RGOF/MoS2 sample could be further optimized by regulating the MoS2 content. Therefore, a new and effective strategy was proposed to develop high efficiency MAs with ultra-lightweight, wide band, thin thickness and strong absorption capabilities. (C) 2021 Elsevier Inc. All rights reserved.

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