Intensity dependence of multiply charged atomic ions from argon clusters in moderate nanosecond laser fields

We report the laser intensity dependence of multiply charged atomic ions (MCAIs) Arn+ with 2 <= n <= 8 from argon clusters in focused nanosecond laser fields at 532 nm. The laser field, in the range of 10(11)-10(12) W/cm(2), is insufficient for optical field ionization but is adequate for multiphoton ionization. The MCAI sections of the mass spectra for clusters containing 3700 and 26 000 atoms are dominated by Arn+ with 7 <= n <= 9, extending to Ar14+. While the distributions of the MCAIs remain largely constant throughout the intensity range of the laser, the abundance of Ar+ relative to the abundances of the MCAIs increases dramatically with increasing laser intensity. Consequently, exponential fittings of the yields result in a larger exponent for Ar+ than for MCAIs, and the exponents of MCAIs with 2 <= n <= 8 are similar, with only slight variations for different charge states. The width of the arrival time and, hence, the corresponding kinetic energy of Ar+ also increases with increasing laser intensities, while the width of the arrival time of MCAIs remains constant throughout the range of measurements. These results call for more detailed theoretical investigations in this regime of laser-matter interactions. Published under an exclusive license by AIP Publishing.

Automated summary

The experimental results showed that the relative abundance of Ar+ in the mass spectra of argon clusters increases significantly with increasing laser intensity, while the distribution of MCAIs remains constant. Additionally, the arrival time width of Ar+ increases with laser intensity, in contrast to the MCAIs which exhibit a constant width. These findings indicate the need for further theoretical investigations into the laser-matter interactions in this regime.