4.7 Article

Thermally annealed self-assembled three-dimensional graphene for direct construction of porous flow distributor in polymer electrolyte membrane fuel cell

Journal

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
Volume 46, Issue 74, Pages 36930-36939

Publisher

PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.ijhydene.2021.08.210

Keywords

PEMFC; Porous flow distributor; 3D graphene; Thermal annealing; Advanced boiling method

Funding

  1. Korea Electric Power Corporation [R19XO01-29]
  2. National Research Foundation of Korea [2019R1C1C1006392]
  3. National Research Foundation of Korea [2019R1C1C1006392] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)

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Self-assembled three-dimensional graphene (STG) with improved conductivity through thermal annealing is applied as a flow distributor in fuel cells to enhance performance, showing lower resistance and improved efficiency in single-cell systems.
Self-assembled three-dimensional graphene (STG), which is constructed via advanced boiling method (ABM) has advantages in terms of low-cost, facile procedures, and needless to use any backbone structure. Although the previously developed STG is considered as a promising material and structure to be used as a flow distributor in polymer electrolyte membrane fuel cell (PEMFC), the STG flow distributor should be advanced in the aspect of conductivity to achieve higher performance. Herein, the conductivity of STG is improved via the thermal annealing process and the advanced STG is applied in PEMFC as a flow distributor to enhance the performance of the single-cell system. Single cell constructed with the thermally annealed STG exhibits a lowered charge and ohmic resistance, which leads to the performance enhancement. These results imply that direct coating of the advanced STG can be one of the alternatives of the complex and high-cost process of graphene coating to the porous metal foam through chemical vapor deposition (CVD). (c) 2021 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.

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