4.7 Article

Superhydrophobic MXene based fabric composite for high efficiency solar desalination

Journal

DESALINATION
Volume 524, Issue -, Pages -

Publisher

ELSEVIER
DOI: 10.1016/j.desal.2021.115475

Keywords

Solar interface desalination; MXene; Emulsion dipping; Super hydrophobic; Salt-resistant

Funding

  1. Natural Science Foundation of China [51873178, 21673203]
  2. Opening Project of State Key Laboratory of Polymer Materials Engineering (Sichuan University) [sklpme2020-4-03]
  3. Qing Lan Project of Yangzhou University
  4. Qing Lan Project of Jiangsu Province
  5. High-end Talent Project of Yangzhou University
  6. Priority Academic Program Development of Jiangsu Higher Education Institutions
  7. Postgraduate Research & Practice Innovation Program of Jiangsu Province [KYCX18_2364, KYCX20_2977]
  8. Outstanding Doctoral Dissertation Fund of Yangzhou University

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This study proposes a new strategy to fabricate a superhydrophobic fabric composite for high-efficiency solar desalination and oil-water separation. The obtained fabric composite is able to prevent salt accumulation even in high salinity conditions and exhibits a high solar interfacial evaporation rate and efficiency.
Solar desalination via interfacial evaporation is an effective, green and convenient method to solve the shortage of fresh water. It remains challenging to develop high quality light absorber materials that can both reduce the heat loss and avoid salt accumulation during the seawater evaporation and be also used in different harsh conditions. Here, we, for the first time, propose an emulsion dip-coating strategy to fabricate a superhydrophobic fabric composite for high-efficiency interfacial evaporation. During the dip-coating in the oil-in-water emulsion, MXene in the water phase together with the polydimethylsiloxane in the oil phase is decorated onto the poly dopamine modified elastic fabric through the interfacial hydrogen bonding. The obtained superhydrophobic/ superoleophilic fabric composite is able to separate the oil from the polluted seawater. Air bubbles are trapped between the fabric and water, reducing the heat conduction to bulk water. Furthermore, the salt is prevented from accumulation on the fabric surface even in a very high salinity condition. The solar interfacial evaporation rate and efficiency reach 1.526 kg m(-2) h(-1) and 93.3% under 1 sun, respectively, and can be almost maintained after a long-time use. This study provides a new avenue to prepare multifunctional light absorbers for efficiency solar desalination and oil-water separation.

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