Journal
DALTON TRANSACTIONS
Volume 51, Issue 10, Pages -Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/d1dt04388a
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Funding
- National Key Research and Development Program Nanotechnology Specific Project [2020YFA0210900]
- National Natural Science Foundation of China [21908255, 22078371, 22108315, 21938001, 21961160741]
- Guangdong Provincial Key RD Programme [2019B110206002]
- Special Fund for Local Science and Technology Development by the Central Government, Local Innovative and Research Teams Project of Guangdong Pearl River Talents Program [2017BT01C102]
- NSF of Guangdong Province [2020A1515011141]
- Science and Technology Key Project of Guangdong Province, China [2020B010188002]
- Basic and Applied Basic Research Program of Guangzhou City [202102020461]
- Guangdong Basic and Applied Basic Research Foundation [2020A1515110864]
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A nitrogen-doped carbon-supported ultrahigh-loading single-site Zn catalyst (Zn-1-N-C, 28.3 wt%) was easily constructed using a ball milling strategy. The catalyst, with atomically dispersed ZnN3O sites, exhibited superior catalytic properties for H-2 generation from silane/alcohol pairs, and scale-up and recycling tests showcased its significant potential in practical applications.
A nitrogen-doped carbon-supported ultrahigh-loading single-site Zn catalyst (Zn-1-N-C, 28.3 wt%) was facilely constructed by using a ball milling strategy. With atomically dispersed ZnN3O sites, the catalyst showed superior catalytic properties for the generation of H-2 from silane/alcohol pairs, and scale-up and recycling tests demonstrated its great potential in practical applications.
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