Journal
CORROSION SCIENCE
Volume 193, Issue -, Pages -Publisher
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.corsci.2021.109899
Keywords
thermal barrier coatings; CMAS corrosion; doped Gd2Zr2O7; first-principles calculation; interface characteristics
Funding
- National Natural Science Foundation of China [51971156, 51801008]
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A CMAS resistant TBC of Sc doped Gd2Zr2O7/YSZ has been developed, which has a higher ability to maintain its lattice structure and coating microstructure under CMAS conditions, alleviating coating degradation.
YSZ thermal barrier coatings (TBCs) are vulnerable to calcium-magnesium-alumina-silicate (CMAS) attack, and a CMAS resistant TBC of Sc doped Gd2Zr2O7/YSZ are developed in this study. At 1250 degrees C, corrosion products form a reaction layer at the CMAS/coating interface, which largely suppresses CMAS further infiltration. Compared with Gd2Zr2O7, Sc doped Gd2Zr2O7 has a higher ability to keep its lattice structure in the presence of CMAS, which is beneficial to maintain the coating microstructure under CMAS conditions, alleviating the coating degradation. First-principles calculation was conducted to investigate the corrosion products formation mechanisms, and the characteristics of CMAS/reaction layer and reaction layer/coating interfaces.
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