Journal
CHEMICAL RECORD
Volume 22, Issue 4, Pages -Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/tcr.202100276
Keywords
Lewis base; Phosphine; Tertiary amine; Divergent reaction; Review
Categories
Funding
- National Natural Science Foundation of China [21702189]
- Key scientific and technological project of Henan Province [202102310004]
- Zhengzhou University [JC21253007]
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Lewis base catalysis provides powerful synthetic strategies for the selective construction of carbon-carbon and carbon-heteroatom bonds. The nucleophilicity and steric hindrance of Lewis base catalyst often plays a major role in catalytic reactivity and selectivity in the reaction. Tremendous progress has been made in the divergent construction of valuable motifs under Lewis base catalysis in the past decades.
Lewis base catalysis provides powerful synthetic strategies for the selective construction of carbon-carbon and carbon-heteroatom bonds. Thus continuous efforts have been deployed to develop effective methodologies involving Lewis base catalysis. The nucleophilicity and steric hindrance of Lewis base catalyst often plays a major role in catalytic reactivity and selectivity in the reaction. In the past decades, tremendous progress has been made in the divergent construction of valuable motifs under Lewis base catalysis. In this review, we provide a comprehensive and updated summary of Lewis base-catalysed chemo-, diastereo- and enantiodivergent reaction, as well as the related mechanism will be highlighted in detail.
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