Journal
CHEMICAL COMMUNICATIONS
Volume 58, Issue 17, Pages 2914-2917Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/d1cc06914d
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Funding
- National Key R&D Program of China [2017YFA0403503]
- National Natural Science Foundation of China [11674001, 21803063, 22003060]
- Open fund for Discipline Construction, Institute of Physical Science and Information Technology (Anhui University) [S01003103]
- Recruitment Program for Leading Talent Team of Anhui Province [LTIT20200002]
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High curvature carbon-supported isolated NiN4 sites with excellent CO2 reduction reaction performance were achieved through a top-down strategy. The charge polarization induced by the axial asymmetry of the carbon substrate enhances COOH* adsorption and reduces the free energy barrier of the rate-determining step.
High curvature carbon-supported isolated NiN4 sites with ideal CO2 reduction reaction performance were obtained through a top-down strategy. The charge polarization induced by the axial asymmetry of the carbon substrate can enhance the adsorption of COOH* and reduce the free energy barrier of the rate-determining step.
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