Journal
CATALYSIS COMMUNICATIONS
Volume 162, Issue -, Pages -Publisher
ELSEVIER
DOI: 10.1016/j.catcom.2021.106382
Keywords
Hydrogen evolution reaction; Transition metal phosphides; Performance; Seawater electrolysis
Categories
Funding
- Key Research and Development Project of Hainan Province [ZDYF2020037, 2020207]
- National Natural Science Foundation of China [21805104]
- Basic and Applied Basic Research Foundation of Guangdong Province [2019A1515110558]
- Start-up Research Foundation of Hainan University (KYQD) [KYQD(ZR)- 20082, KYQD(ZR)-20083, KYQD(ZR)-20084, KYQD(ZR)-21065]
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This review provides a brief introduction to the reaction mechanism of seawater electrocatalytic process and evaluates recent progress in transition metal phosphides-based catalysts for seawater electrolysis. The challenges and opportunities of transition metal phosphides are also discussed.
The electrocatalytic seawater splitting has become an important and necessary way for large-scale hydrogen production with challenges ahead. In this review, a brief introduction to the reaction mechanism of seawater electrocatalytic process is first provided, including the cathodic hydrogen evolution reaction and the anodic oxygen evolution reaction, as well as the competitive chloride evolution reaction. Recent progress in transition metal phosphides-based catalysts for seawater electrolysis, such as phosphorus doped transition metals, binary metal phosphides, and structural engineering are then evaluated and discussed. Finally, the challenges and opportunities of transition metal phosphides are proposed and discussed.
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