4.7 Article

Anisotropic optical gains in α-plane ZnO/Zn0.8Mg0.2O multiple quantum wells grown via pulsed-laser deposition

Journal

APPLIED SURFACE SCIENCE
Volume 565, Issue -, Pages -

Publisher

ELSEVIER
DOI: 10.1016/j.apsusc.2021.150401

Keywords

ZnO; ZnMgO MQWs; Amplified spontaneous emission; Degree of polarization; Characteristic temperature

Funding

  1. Ministry of Science and Technology of Taiwan [MOST 1092112-M-027-001-, MOST 110-2112-M-027-006-]

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High periodicity non-polar ten-pair ZnO/Zn0.8Mg0.2O multiple quantum wells were prepared via pulsed-laser deposition on r-plane sapphire, demonstrating anisotropic optical properties with energy difference between splitting valence bands. The amplified spontaneous emission from the non-polar MQWs showed higher efficiency under perpendicular pump condition, with linearly polarized ASE and dominant ex-ex scattering mechanism. The temperature-dependent ASE revealed red shift in emission peak and a temperature-insensitive characteristic temperature of -124 K.
High periodicity non-polar ten-pair ZnO/Zn0.8Mg0.2O multiple quantum wells (MQWs), with a binding energy of approximately 69.8 meV, on r-plane sapphire were prepared via pulsed-laser deposition. The a-plane ZnO/ Zn0.8Mg0.2O MQWs exhibit anisotropic optical properties, which demonstrate an energy difference of approximately 15 meV between the two splitting valence bands via photoluminescence measurement. Through the optical pump of the Q-switched laser, the amplified spontaneous emission (ASE) from both the side and surface normal of the non-polar MQWs shows a higher slope efficiency and gain coefficient under a perpendicular pump (Epic) than those under a parallel pump condition (Ep//c). Owing to the gain-guiding effect, the linealy polarized ASE from the side of the non-polar ZnO/Zn0.8Mg0.2O MQWs has been demonstrated with a degree of polarization (DOP) - 89 %. For the surface normal ASE, the P2 band emission from exciton-exciton (ex-ex) scattering is recognized as the dominant mechanism. Through the temperature-dependent ASE, the P band emission peak reveals an evident red shift as the temperature increases. Moreover, a higher characteristic temperature of - 124 K, which indicates the temperature-insensitive property, is obtained.

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