Journal
APPLIED SURFACE SCIENCE
Volume 565, Issue -, Pages -Publisher
ELSEVIER
DOI: 10.1016/j.apsusc.2021.150444
Keywords
Bi2O2S; Photoelectrochemical; Photodetector; Self-healing
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Funding
- Open Fund based on innovation platform of Hunan colleges and universities [19K095]
- National Natural Science Foundation of China [11874316]
- Program for Changjiang Scholars and Innovation Research Team in University [IRT 17R91]
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In this study, a high-performance photodetector based on Bi2O2S nanoplates was developed, demonstrating excellent optical response switching behaviors and long-term stability, as well as showing self-healing properties in alkaline environments.
Sulfur oxygen bismuth (Bi2O2S), as a newly emerging two-dimensional material in the domain of optoelectronics, was increasingly concerned by researchers due to its high carrier lifetime and unique loose structure. Herein, we built a photoelectrochemical (PEC) type photodetectors (PDs) based Bi2O2S nanoplates exhibiting the excellent optical response switching behaviors with the high responsivity (2.31 mA/W) at 0.6 V potential and the rapid response time (similar to 0.08 s), as well as the great long-term stability and durability (over one month). Meanwhile, we demonstrated the self-healing properties in alkaline by testing the open-circuit potential (OCP) time profile. The lifetime of photo-generated carriers can be extended in this process, which in turn enables the detector to operate for a long time. In this way, the PDs based Bi2O2S nanoplates enriched its basic research in the field of photo-electrochemical and paved the way for the research of energy storage devices.
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