4.6 Article

Role of magnetocrystalline anisotropy on anisotropic magnetocaloric effect in single crystals

Journal

APPLIED PHYSICS LETTERS
Volume 119, Issue 21, Pages -

Publisher

AIP Publishing
DOI: 10.1063/5.0068818

Keywords

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Funding

  1. National Natural Science Foundation of China [11774045]
  2. Joint Research Fund Liaoning-Shenyang National Laboratory for Materials Science [20180510008]
  3. Fundamental Research Funds for Central Universities [N2102006]

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The role of magnetocrystalline anisotropy in single crystals on the anisotropic magnetocaloric effect was studied using Monte Carlo simulation. The study found that anisotropy can affect the spin reorientation transition temperature and the magnetization behavior at low temperatures and weak fields. Additionally, the anisotropy of entropy change is most significant when the magnetic field is parallel to the easy axis.
The role of magnetocrystalline anisotropy in single crystals played on the anisotropic magnetocaloric effect is studied based on Monte Carlo simulation. By taking into account the anisotropy, the spin reorientation transition (SRT) temperature (T-SRT) may be higher than the Curie temperature and enhanced with larger anisotropy, and the magnetization behaviors at low temperatures below T-SRT and under weak fields are highly sensitive to the anisotropy. The anisotropy of entropy change is the most significant when the magnetic field is parallel to the easy axis, while the maximum entropy change may increase or decrease with the anisotropy constant in a given direction depending on the magnetic field strength. Power-law fits have been conducted on the field dependence of the maximum entropy change and relative cooling power, which not only indicate a characteristic of the second-order phase transition but also demonstrate effect of anisotropy on magnetic order and dynamics during the SRT to contribute to the anisotropic magnetocaloric effect. Published under an exclusive license by AIP Publishing.

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