4.7 Article

Influence of heterogeneities of density on the hydromechanical behaviour of pellet-based bentonite materials in imbibition experiments

Journal

APPLIED CLAY SCIENCE
Volume 216, Issue -, Pages -

Publisher

ELSEVIER
DOI: 10.1016/j.clay.2021.106353

Keywords

Bentonite; Pellet mixture; Imbibition experiment; Swelling pressure; Relative humidity; Water migration

Funding

  1. Ecole des Ponts ParisTech
  2. French National Agency for Radioactive Waste Management (Andra)

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The experimental investigation focused on the hydromechanical behavior of pellet-powder mixtures used for sealing galleries in radioactive waste disposal concepts. Results showed that water vapor flux dominated hydration, with pellets and inter-pellet pores not in hydraulic equilibrium, and the material gradually lost its granular structure during hydration.
An experimental investigation on the hydromechanical behaviour of pellet-powder mixtures, candidate materials for sealing the galleries in radioactive waste disposal concepts, was described. Imbibition experiments were performed using a specially-designed column, with square cross-section and glass sides allowing pictures to be taken by a camera. Relative humidity and swelling pressure were measured at different elevations of the column. Three mixtures with an identical pellet volume fraction and various powder volume fractions were used to study the influence of heterogeneities of density on the hydromechanical behaviour of the mixture under repository conditions. Results demonstrated that hydration of the material was dominated by water vapour flux, with pellets and inter-pellet pores not at hydraulic equilibrium. In mixtures with low powder content, the evolution of swelling pressure was controlled by contact forces between pellets. The material progressively lost the initial granular structure upon hydration. Note that hydration was made by imbibition, instead of injecting liquid water at high pressure, to avoid unrealistic liquid water flow rates in the initial large inter-pellet voids. In addition, sensors four times larger than the pellets were used to measure a representative value of swelling pressure.

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