Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 61, Issue 17, Pages -Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.202200598
Keywords
batteries; cathode materials; zinc batteries
Categories
Funding
- National Natural Science Foundation of China [51972346, 51932011]
- Hunan Outstanding Youth Talents [2021JJ10064]
- Program of Youth Talent Support for Hunan Province [2020RC3011]
- Innovation-Driven Project of Central South University [2020CX024]
- Ministry of Education [RG157/19]
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This review comprehensively summarizes the rational design strategies of high-energy-density zinc batteries, critically analyzes the positive effects and potential issues of these strategies, and outlines the challenges and perspectives for further development.
In recent years, the increasing demand for high-capacity and safe energy storage has focused attention on zinc batteries featuring high voltage, high capacity, or both. Despite extensive research progress, achieving high-energy-density zinc batteries remains challenging and requires the synergistic regulation of multiple factors including reaction mechanisms, electrodes, and electrolytes. In this Review, we comprehensively summarize the rational design strategies of high-energy-density zinc batteries and critically analyze the positive effects and potential issues of these strategies in optimizing the electrochemistry, cathode materials, electrolytes, and device architecture. Finally, the challenges and perspectives for the further development of high-energy-density zinc batteries are outlined to guide research towards new-generation batteries for household appliances, low-speed electric vehicles, and large-scale energy storage systems.
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