Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 61, Issue 8, Pages -Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.202115136
Keywords
Lead-free materials; Low-dimensional perovskites; Luminescence; Manganese; Nanocomposites
Categories
Funding
- National Natural Science Foundation of China [NSFC 51932009, 51772288, 52172166, U2005212, 52072349]
- Chinese Government [2017YFE0132300]
- Australian Government [2017YFE0132300]
- Projects for science and technology development plan of Jilin province [20210402046GH]
- Open Funds of the State Key Laboratory of Rare Earth Resource Utilization [RERU2020005]
- Natural Science Foundation of Zhejiang Province [LR22E020004]
- Science and Technology Innovation Commission of Shenzhen
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This study demonstrates an efficient anticounterfeiting strategy based on dual optical encryption by combining up- and downconversion luminescence in a nanocomposite material. The emission color of the nanocomposite can be changed by varying the excitation source, allowing for different luminescent patterns to improve the anticounterfeiting index and fabricate professional anticounterfeiting materials.
In view of their excellent luminescence properties, nanocrystalline metal halide perovskites have diverse optoelectronic applications, including those related to anticounterfeiting. However, high-quality optical anticounterfeiting typically requires multiple encryptions relying on several optical modes to ensure information security. Herein, an efficient anticounterfeiting strategy based on dual optical encryption is realized by combining up- and downconversion luminescence in a nanocomposite with NaYF4 : Er3+,Yb3+ as core and a CsMnCl3 as shell. The emission color of this nanocomposite depends on the penetration depth of incident radiation and can be changed by varying the excitation source (980 nm laser or UV light) to produce different luminescent patterns. This feature allows one to effectively improve the anticounterfeiting index and fabricate professional anticounterfeiting materials.
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