4.8 Article

Ultrahigh Sensitive Au-Doped Silicon Nanomembrane Based Wearable Sensor Arrays for Continuous Skin Temperature Monitoring with High Precision

Journal

ADVANCED MATERIALS
Volume 34, Issue 4, Pages -

Publisher

WILEY-V C H VERLAG GMBH
DOI: 10.1002/adma.202105865

Keywords

epidermal electronics; gold-doped silicon nanomembranes; high-precision thermal monitoring

Funding

  1. National Research Foundation of Korea [NRF-2018M3A7B4071109, NRF-2019R1A2C2086085, NRF-2021R1A4A1031437, NRF-2019R1A6A1A11055660]
  2. National Research Foundation of Korea (NRF) - Ministry of Science and ICT [NRF-2017M3A7B4049466]
  3. KIST Institutional Program [2Z06430-20-P064]
  4. R&D program of MOTIE/KEIT [20012460]
  5. Korea Medical Device Development Fund - Korea government (the Ministry of Science and ICT) [KMDF_PR_20200901_0093, 9991006766]
  6. National Research Foundation of Korea (NRF) - Ministry of Science [NRF-2020R1C1C1013900]
  7. IEN Center Grant (Center for Human-Centric Interfaces and Engineering) from the Georgia Tech Institute for Electronics and Nanotechnology
  8. Korea Evaluation Institute of Industrial Technology (KEIT) [20012460] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
  9. National Research Foundation of Korea [2018M3A7B4071109, 2019R1A6A1A11055660] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)

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This study introduces a new type of ultrasensitive and stretchable gold-doped silicon nanomembrane epidermal temperature sensor array, which shows high thermal sensitivity and scalability for continuous monitoring of body temperature and respiration rate. The technology has the potential for precision diagnosis and disease management.
Monitoring the body temperature with high accuracy provides a fast, facile, yet powerful route about the human body in a wide range of health information standards. Here, the first ever ultrasensitive and stretchable gold-doped silicon nanomembrane (Au-doped SiNM) epidermal temperature sensor array is introduced. The ultrasensitivity is achieved by shifting freeze-out region to intrinsic region in carrier density and modulation of fermi energy level of p-type SiNM through the development of a novel gold-doping strategy. The Au-doped SiNM is readily transferred onto an ultrathin polymer layer with a well-designed serpentine mesh structure, capable of being utilized as an epidermal temperature sensor array. Measurements in vivo and in vitro show temperature coefficient of resistance as high as -37270.72 ppm degrees C-1, 22 times higher than existing metal-based temperature sensors with similar structures, and one of the highest thermal sensitivity among the inorganic material based temperature sensors. Applications in the continuous monitoring of body temperature and respiration rate during exercising are demonstrated with a successful capture of information. This work lays a foundation for monitoring body temperature, potentially useful for precision diagnosis (e.g., continuous monitoring body temperature in coronavirus disease 2019 cases) and management of disease relevance to body temperature in healthcare.

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