4.8 Article

All-Solid-State Vertical Three-Terminal N-Type Organic Synaptic Devices for Neuromorphic Computing

Journal

ADVANCED FUNCTIONAL MATERIALS
Volume 32, Issue 21, Pages -

Publisher

WILEY-V C H VERLAG GMBH
DOI: 10.1002/adfm.202107314

Keywords

neuromorphic computing; n-type conjugated polymers; n-type organic synaptic devices; synaptic transistors

Funding

  1. National Natural Science Foundation of China [61874051, U1732136]
  2. Key Program of Natural Science Foundatio of Gansu Province [20JR5RA296]
  3. Supercomputing Center of Lanzhou university

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This study introduces a novel n-type organic artificial synaptic device that achieves high current density operation and mimics the basic functions of biological synapses. It shows excellent energy consumption performance and simulation results demonstrate a recognition accuracy of 94%.
Artificial synaptic devices are the basic composition units for neuromorphic computing processors that realize massive parallel computing. However, the n-type organic transistors have failed to achieve good performance as an artificial synaptic device for neuromorphic computing until now. Here, a vertical three-terminal n-type organic artificial synapse (TNOAS) using a lithium ion-based organic dielectric and the n-type donor-acceptor (D-A) conjugated polymer-naphthalene-1,4,5,8-tetracarboxylic-diimide-thiophene-vinyl-thiophene (NDI-gTVT) as the channel is proposed. The TNOAS achieves nonvolatile conductance modulation with high current density operation (approximate to 10 KA cm(-2)) at low voltage and mimics the basic functions of biological synapses, such as long-term synaptic plasticity and paired-pulse facilitation. The minimum energy consumption of a response event triggered by a single action potential is 6.16 pJ, which can be comparable with p-type counterparts. Moreover, simulation using handwritten digital datasets exhibit a high recognition accuracy of 94%.

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