4.8 Article

InAsP Quantum Dot-Embedded InP Nanowires toward Silicon Photonic Applications

Journal

ACS APPLIED MATERIALS & INTERFACES
Volume 14, Issue 10, Pages 12488-12494

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acsami.1c21013

Keywords

quantum dot-embedded nanowire; InAsP quantum dot; VLS epitaxy; silicon photonics; exciton-biexciton transition

Funding

  1. National Science Foundation [ECCS-1810548]
  2. Institute for Information & Communications Technology Promotion (IITP)
  3. National Research Foundation of Korea (NRF) - Korea government (MSIT) [20170000740011001, NRF-2017R1E1A1A01075263]

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This article reports on the monolithic integration of InAsP quantum dots embedded in InP nanowires on silicon, showing potential for building next-generation quantum light sources.
Quantum dot (QD) emitters on silicon platforms have been considered as a fascinating approach to building next-generation quantum light sources toward unbreakable secure communications. However, it has been challenging to integrate position-controlled QDs operating at the telecom band, which is a crucial requirement for practical applications. Here, we report monolithically integrated InAsP QDs embedded in InP nanowires on silicon. The positions of QD nanowires are predetermined by the lithography of gold catalysts, and the 3D geometry of nanowire heterostructures is precisely controlled. The InAsP QD forms atomically sharp interfaces with surrounding InP nanowires, which is in situ passivated by InP shells. The linewidths of the excitonic (X) and biexcitonic (XX) emissions from the QD and their powerdependent peak intensities reveal that the proposed QD-in-nanowire structure could be utilized as a non-classical light source that operates at silicon-transparent wavelengths, showing a great potential for diverse quantum optical and silicon photonic applications.

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