Journal
ACS APPLIED MATERIALS & INTERFACES
Volume 13, Issue 41, Pages 48795-48800Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acsami.1c14505
Keywords
E-fuel; passive fuel cell; current collector design; power density; long-term stability; hydrogen evolution
Funding
- Research Grant Council of the Hong Kong Special Administrative Region, China [T23-601/17-R]
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Passive fuel cells that use diffusion and natural convection for fuel delivery are considered promising for powering portable devices, while those using typical liquid alcohol fuels still face performance limitations that hinder commercialization. The introduction of electrically rechargeable liquid fuel (e-fuel) as a novel concept has drawn attention for its rechargeability, cost-effectiveness, and superior reactivity. A passive fuel cell using e-fuel and ambient air for electricity production has been designed and shown to achieve a peak power density of 116.2 mW cm(-2) and stable operation for over 350 hours, indicating great potential for future applications.
Passive fuel cells, using diffusion and natural convection for fuel delivery, are regarded as promising candidates for powering portable devices including mobile phones and laptops. However, the performance of passive fuel cells which employ typical liquid alcohol fuels are still limited, which thereby greatly hampered their commercialization progress. Recently, a novel concept named the electrically rechargeable liquid fuel (e-fuel), with its rechargeability, cost-effectiveness, and superior reactivity, has attracted increasing attention. In this study, a passive fuel cell using the liquid e-fuel and the ambient air for electricity production is designed and fabricated. This passive fuel cell is demonstrated to achieve a peak power density of 116.2 mW cm(-2) along with a stable operation for over 350 h, exhibiting great prospect for future applications.
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