Journal
JOURNAL OF POLYMER SCIENCE
Volume 60, Issue 6, Pages 865-916Publisher
WILEY
DOI: 10.1002/pol.20210592
Keywords
emerging photovoltaics; energy level regulation; organometallic complexes; p-dopant additives
Categories
Funding
- National Natural Science Foundation of China [22005024, 51961165102, 51873007, 21835006, 52003022]
- Fundamental Research Funds for the Central Universities [PT2021-02, buctrc202009]
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Organometallic complexes (OMCs) with organic and metal active moieties show great potential in solar cells, providing diverse structures and unique charge centers for improved performance. They can be used as active or interlayer materials in various solar cell systems, using some metals as dopants to enhance photoelectric performance. Opportunities and challenges of OMCs in solar cell applications are discussed.
Organometallic complexes (OMCs) consisting of organic and metal active moieties have shown immense potential for application in solar cells. The diverse structure, rich porosity, and unique charge centers of OMCs enable them to be functional in solar cells. In this review, we introduced four types of OMCs, such as crown organometallic complexes, beta-diketone metal complexes, cyclometallic complexes, and main chain metal-containing polymers, providing an in-depth analysis of the structure-performance relationship. OMCs could serve as active or interlayer materials in a variety of solar cell systems such as organic solar cells, perovskite solar cells, and dye-sensitized solar cells, especially some metals to improve the photoelectric performance of the device as dopants. In the end, perspectives on the opportunities and challenges of OMCs are given.
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