Journal
JOURNAL OF MATERIOMICS
Volume 8, Issue 1, Pages 1-8Publisher
ELSEVIER
DOI: 10.1016/j.jmat.2021.06.006
Keywords
G-C3N4; NO removal; Oxygen vacancies; Photocatalysis; S-scheme
Funding
- Vietnam National Foundation for Science and Technology Development (NAFOSTED) [103.02-2019.343]
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This report investigates the performance of SnO2-x/g-C3N4 heterojunction photocatalyst in the photocatalytic degradation of NO. The results show that this hybrid photocatalyst has higher NO degradation efficiency and selectivity compared to g-C3N4, and it also exhibits good stability. This study is of great significance for the development of efficient environmental treatment materials.
NOx emissions cause many negative impacts on the living environment. The photocatalysis of semiconductors is superior for nitric oxide (NO) degradation due to their low redox potential. In this report, we combine SnO2-x/g-C3N4 heterojunction photocatalyst toward the high selectivity into green products under visible light illumination. Results show that SnO2-x/g-C3N4 heterojunction degraded 40.8% of NO, which is 1.6 times higher than that of g-C3N4. In addition, the selectivity coefficient of SnO2-x/g-C3N4 is higher 3 times than both pure SnO2, and g-C3N4. Furthermore, SnO2-x/g-C3N4 expresses a superior stability for NO photocatalytic-degradation after five cycles. The scavenger trapping test results, and electron spin resonance (ESR) analysis also provide more understanding of the charge transfer mechanism of materials. SnO2-x/g-C3N4 heterojunction shows a high removal efficiency of NO gas, making it an up-and-coming environmental treatment candidate. (C) 2021 The Chinese Ceramic Society. Production and hosting by Elsevier B.V.
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