4.6 Article

Modeling of Spherical Dust Particle Charging due to Ion Attachment

Journal

FRONTIERS IN EARTH SCIENCE
Volume 9, Issue -, Pages -

Publisher

FRONTIERS MEDIA SA
DOI: 10.3389/feart.2021.709890

Keywords

dust particle electrification; dust particle charging; ion attachment; dust particle settling; dust particle transport; atmospheric electricity

Funding

  1. European Union (European Social Fund-ESF) by the Operational Programme Human Resources Development, Education and Lifelong Learning 2014-2020
  2. European Union (European Social Fund-ESF) [MIS-5000432]
  3. project D-TECT - European Research Council (ERC) under the European Union's Horizon 2020 research and innovation programme [725698]
  4. [MIS 5049929]
  5. [EDBM103]

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The study examines the attachment of positive and negative ions to settling spherical dust particles using a novel numerical model. The model calculates the modification of atmospheric ion densities, atmospheric electrical conductivity, and large-scale electric field in the presence of dust particles. While particles can acquire varying amounts of electrical charge and the electric field can increase significantly, the electrical force is not sufficient to significantly influence their gravitational settling.
The attachment of positive and negative ions to settling spherical dust particles is studied. A novel 1D numerical model has been developed to parameterize the charging process in the presence of a large-scale electric field. The model is able to self-consistently calculate the modification of atmospheric ion densities in the presence of the dust particles, and the consequent alteration of the atmospheric electrical conductivity and the large-scale electric field. Moreover, the model estimates the acquired electrical charge on the dust particles and calculates the electrical force that is applied on them. Using observed dust size distributions, we find that the particles can acquire electrical charge in the range of 1-1,000 elementary charges depending on their size and number density. The particles become mainly negatively charged, but under specific conditions giant mode particles (larger than 50 mu m radius) can be positive. Moreover, the large-scale electric field can increase up to 20 times as much as the fair weather value. However, our approach shows that the resultant electrical force is not enough to significantly influence their gravitational settling, as the ratio between the electrical force magnitude and the gravity magnitude does not exceed the value of 0.01. This indicates that the process of ion attachment alone is not sufficient to create strong electrical effects for the modification of particle dynamics. Therefore, other processes, such as the triboelectric effect and updrafts, must be included in the model to fully represent the impact of electricity on particle dynamics.

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