Journal
GEOPHYSICAL RESEARCH LETTERS
Volume 43, Issue 16, Pages 8720-8727Publisher
AMER GEOPHYSICAL UNION
DOI: 10.1002/2016GL070075
Keywords
domestic coal combustion; COS; CO; SO2; emission
Categories
Funding
- Strategic Priority Research Program projects of the Chinese Academy of Sciences [XDB05010100]
- Special Fund for Environmental Research in the Public Interest [201509002]
- National Natural Science Foundation of China [21477142, 41575121, 41203070]
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Carbonyl sulfide (COS), carbon monoxide (CO), and sulfur dioxide (SO2) emissions generated from prevailing domestic coal stoves fueled with raw bituminous coal were studied under alternation cycles of flaming and smoldering combustion. The measurements in the laboratory and the farmer's house indicated that COS and CO emissions mainly occurred under the condition of flame extinguishment after coal loading, whereas SO2 emissions were mainly generated through combustion with flame. The COS emission factors for the domestic stoves in the laboratory and the farmer's house were recorded as 0.570.10gCOSkg(-1) and 1.430.32gCOSkg(-1), being approximately a factor of 50 and 125 greater than that generated from coal power plants, respectively. Based on the COS emission factors measured in this study, COS emission from only domestic coal combustion in China would be at least 30.55.6GgSyr(-1) which was 1 magnitude greater than the current COS estimation from the total coal combustion in China.
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