4.7 Article

High-performance Ba1-xKxFe2As2 superconducting tapes with grain texture engineered via a scalable fabrication

Journal

SCIENCE CHINA-MATERIALS
Volume 64, Issue 10, Pages 2530-2540

Publisher

SCIENCE PRESS
DOI: 10.1007/s40843-020-1643-1

Keywords

iron-based superconductors; critical current density; scalable; grain texture; hot isostatic pressing

Funding

  1. National Key RAMP
  2. D Program of China [2018YFA0704200, 2017YFE0129500]
  3. National Natural Science Foundation of China [51861135311, U1832213, 51721005]
  4. Strategic Priority Research Program of Chinese Academy of Sciences [XDB25000000]
  5. Key Research Program of Frontier Sciences of Chinese Academy of Sciences [QYZDJ-SSW-JSC026]

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The development of high-field magnets relies heavily on the performance of superconducting materials. Iron-based superconductors show promise for high-field applications, with Cu/Ag composite-sheathed Ba122 superconducting tapes achieving practical-level critical current density. By manipulating grain texture through rolling and densification, the transport properties of the tapes can be enhanced.
Nowadays the development of high-field magnets strongly relies on the performance of superconducting materials. Iron-based superconductors (IBSs) exhibit high upper critical fields and low electromagnetic anisotropy, making them particularly attractive for high-field applications, especially in particle accelerator magnets, nuclear magnetic resonance spectrometers, medical magnetic resonance imaging systems and nuclear fusion reactors. Herein, through an industrially scalable manufacturing strategy, a practical-level critical current density up to 1.1x10(5) A cm(-2) at 4.2 K in an external magnetic field of 10 T was achieved in Cu/ Ag composite-sheathed Ba1-xKxFe2As2 (Ba122) superconducting tapes. The preparation strategy combines flat rolling to induce grain texture and subsequent hot-isostaticpressing densification. By varying the parameters of rolling, the degree of grain texture was engineered. It is found that the transport properties of the Ba122 tapes can be enhanced by applying a large amount of deformation during rolling, which can be attributed to the improved degree of c-axis texture. Microstructure characterizations on the highest-performance tape demonstrate that the Ba122 phase has a uniform element distribution and small grains with good connectivity. Grain boundary pinning is consequently enhanced as proved by large currents circulating through the sample even at 25 K. Our work proves that Cu/Ag composite-sheathed Ba122 superconducting tapes can be a promising competitor for practical high-field applications in terms of the viable, scalable and cost-effective fabrication strategy applied and the high transport properties achieved in this work.

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