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Preparation, Characterization of Graphitic Carbon Nitride Photo-Catalytic Nanocomposites and Their Application in Wastewater Remediation: A Review

Journal

CRYSTALS
Volume 11, Issue 7, Pages -

Publisher

MDPI
DOI: 10.3390/cryst11070723

Keywords

graphite carbon nitride nanocomposites; photocatalysts; wastewater; computational simulation; artificial intelligence

Funding

  1. Guizhou Science and Technology Support Plan Project [[2019] 1217]
  2. China Postdoctoral Science Foundation [2020M673582XB]
  3. Guizhou Forestry Research [[2017] 17]
  4. Guizhou Science and Technology [[2017] 7371]

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Carbon nitride is a promising material for addressing energy and environmental issues, with good stability and chemical structure, and wide application in the field of photocatalysis.
Energy crisis and environmental pollution are the major problems of human survival and development. Photocatalytic technology can effectively use solar energy and is prospective to solve the above-mentioned problems. Carbon nitride is a two-dimensional polymer material with a graphite-like structure. It has good physical and chemical stabilities, unique chemical and electronic energy band structures, and is widely used in the field of photocatalysis. Graphitic carbon nitride has a conjugated large pi bond structure, which is easier to be modified with other compounds. thereby the surface area and visible light absorption range of carbon nitride-based photocatalytic composites can be insignificantly increased, and interface electron transmission and corresponding photogenerated carriers separation of streams are simultaneously promoted. Therefore, the present study systematically introduced the basic catalytic principles, preparation and modification methods, characterization and calculation simulation of carbon nitride-based photocatalytic composite materials, and their application in wastewater treatment. We also summarized their application in wastewater treatment with the aid of artificial intelligence tools. This review summarized the frontier technology and future development prospects of graphite phase carbon nitride photocatalytic composites, which provide a theoretical reference for wastewater purification.

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