Universal Structural Influence on the 2D Electron Gas at SrTiO3 Surfaces

The 2-dimensional electron gas (2DEG) found at the surface of SrTiO3 and related interfaces has attracted significant attention as a promising basis for oxide electronics. In order to utilize its full potential, the response of this 2DEG to structural changes and surface modification must be understood in detail. Here, a study of the detailed electronic structure evolution of the 2DEG as a function of sample temperature and surface step density is presented. By comparing the experimental results with ab initio calculations, it is shown that local structure relaxations cause a metal-insulator transition of the system around 135 K. This study presents a new and simple way of tuning the 2DEG via surface vicinality and identifies how the operation of prospective devices will respond to changes in temperature.

Automated summary

This study investigates the evolution of the electronic structure of a 2-dimensional electron gas (2DEG) on SrTiO3 surfaces, showing a metal-insulator transition around 135 K caused by local structure relaxations. The research presents a new method of tuning the 2DEG via surface vicinality and explores how prospective devices will respond to temperature changes through experimental and theoretical comparisons.