Surface Lattice Resonances in Self-Templated Plasmonic Honeycomb and Moire Lattices

Surface lattice resonances appear in periodic plasmonic nanoparticle arrays due to the hybridization of plasmonic and photonic modes. Compared to localized surface plasmon resonances of single particles, these coupled modes feature reduced linewidth, angle-dependent dispersion, and long-range collectivity. Here, the optical response of self-assembled plasmonic monolayers of periodically arranged gold and silver nanoparticles is studied. In comparison to already established hexagonal lattices, self-templated honeycomb and Moire type lattices as well as their binary counterparts that include silver and gold nanoparticles in the same monolayer are looked at. All periodic arrays feature macroscopic dimensions (cm-scale) and support surface lattice resonances as evidenced from classical extinction measurements. The experimental findings are supported by results from finite difference time domain simulations. Variation of the plasmonic material, the lattice spacing, and geometry enables spectral tunability of the optical response of the lattices.

Automated summary

Surface lattice resonances in periodic plasmonic nanoparticle arrays are influenced by the hybridization of plasmonic and photonic modes, leading to reduced linewidth, angle-dependent dispersion, and long-range collectivity compared to localized surface plasmon resonances. The optical response of self-assembled plasmonic monolayers of gold and silver nanoparticles with different lattice arrangements is studied in this research, showcasing the spectral tunability of the optical response through variations in plasmonic material, lattice spacing, and geometry. Experimental findings confirming surface lattice resonances are supported by finite difference time domain simulations.