4.6 Article

Probing Transient Localized Electromagnetic Fields Using Low- Energy Point-Projection Electron Microscopy

Journal

ACS PHOTONICS
Volume 8, Issue 9, Pages 2573-2580

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acsphotonics.1c00775

Keywords

ultrafast electron microscopy; streaking spectroscopy; point-projection electron microscopy; surface plasmon polaritons; adiabatic nanofocusing; charge dynamics

Funding

  1. Deutsche Forschungsgemeinschaft within the Priority Program QUTIF [SPP1840]
  2. German-Israeli Foundation (GIF Grant) [1256]
  3. Korea Foundation for International Cooperation of Science and Technology (Global Research Laboratory project) [K20815000003]
  4. Studienstiftung des Deutschen Volkes
  5. [SPP1839]

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The use of low kinetic energy electrons in ultrafast electron microscopy techniques allows for probing nanoscale dynamic processes with reduced radiation doses and enhanced interaction with confined electromagnetic fields. Recent advancements in spatial and temporal resolution have been achieved by combining nanotip photoemitters and point-projection imaging schemes. This enables the analysis of low-energy electron interaction with transient electric fields and opens up possibilities for characterizing vectorial near-fields through electron streaking spectroscopy.
Low kinetic energy electrons are of interest for probing nanoscale dynamic processes using ultrafast electron microscopy techniques. Their low velocities reduce radiation doses and enhance the interaction with confined electromagnetic fields and, thus, may enable ultrafast spectroscopy of single nanostructures. Recent improvements in the spatial and temporal resolution of ultrafast, low-energy electron microscopy have been achieved by combining nanotip photoemitters and point-projection imaging schemes. Here, we use such an ultrafast point-projection electron microscope (UPEM) to analyze the interaction of low-energy electrons with transient electric fields created by photoemission from a nanogap antenna. By analyzing their kinetic energy distribution, we separate angular deflection due to radial field components from electron energy gain and loss due to their axial acceleration. Our measurements open up a route toward the spatial and temporal characterization of vectorial near-fields by low energy electron streaking spectroscopy.

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