4.6 Article

Hybrid Plasmonic Surface Lattice Resonance Perovskite Lasers on Silver Nanoparticle Arrays

Journal

ADVANCED OPTICAL MATERIALS
Volume 9, Issue 17, Pages -

Publisher

WILEY-V C H VERLAG GMBH
DOI: 10.1002/adom.202100299

Keywords

hybrid plasmonic mode; perovskites; strong light-matter interaction; surface lattice resonance

Funding

  1. Ministry of Education (MOE) in Taiwan
  2. [MOST 109-2124-M-009-005]
  3. [MOST 109-2221-E-009-150]
  4. [MOST 107-2221-E-009-116-MY3]
  5. [MOST 108-2112-M-001-044-MY2]

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The research demonstrates a hybrid plasmonic surface lattice resonance (SLR) laser constructed by a MAPbBr(3) perovskite thin film on an Ag nanoparticle array, with high refractive index of the film leading to high spontaneous emission coupling factor and low threshold lasing. The spin-coating process used to grow the perovskite thin film leaves air gaps underneath, providing a large index difference in the periodic array, beneficial for laser operation. The lasing behaviors of the hybrid plasmonic SLR perovskite laser exhibit excellent characteristics, with fixed polarization, enhancing lasing performance and enabling low-cost, low-energy-consumption laser applications.
The hybrid plasmonic surface lattice resonance (SLR) laser constructed by a MAPbBr(3) perovskite thin film on the Ag nanoparticle array is unambiguously demonstrated in this research. The relatively high refractive index of the perovskite thin film provides an excellent coupling between the photonic mode and SLR, leading to a high spontaneous emission coupling factor and a low threshold lasing. Furthermore, a novel spin-coating process applied to grow the MAPbBr(3) perovskite thin film can leave air gaps under the perovskite that provides a large index difference in the periodic array, making the hybrid plasmonic SLR exhibits a high density of state, which is beneficial for laser operation. Via theoretical design and experimental verification, the lasing behaviors of the hybrid plasmonic SLR perovskite laser show excellent characteristics with a fixed polarization. This demonstration facilitates an enhanced lasing performance and realization of the low-cost and low-energy-consumption laser application.

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