4.2 Article

FeS2 encapsulated with mesoporous carbon for high-performance lithium-ion batteries

Journal

MRS COMMUNICATIONS
Volume 11, Issue 4, Pages 418-424

Publisher

SPRINGER HEIDELBERG
DOI: 10.1557/s43579-021-00048-6

Keywords

Composite; Energy storage; Microstructure; Morphology

Funding

  1. National Natural Science Foundation of China [51771145]
  2. China Postdoctoral Science Foundation [2020T130525]
  3. Shaanxi Province Postdoctoral Science Foundation [2018BSHEDZZ113]
  4. ISF-NSFC Joint Research Program [51961145305]
  5. Shaanxi Natural Science Basic Research Plan, China [2020JM-464]

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A strategy of introducing mesoporous carbon (MPC) to obtain a FeS2/MPC composite electrode for lithium-ion batteries (LIBs) was proposed in this study, resulting in a significant improvement in electrochemical performance compared to pristine FeS2. The discharge capacity of the composite electrode reached 650 mAh g(-1) at 0.5 C current density, demonstrating its potential for practical applications.
FeS2 is thought to be a kind of promising anode materials used for lithium-ion batteries (LIBs), but the intrinsic low electrical conductivity and remarkable volume change hinder its practical application. In the present work, we proposed a strategy by introducing mesoporous carbon (MPC) to obtain a FeS2/MPC composite electrode for LIBs. The FeS2/MPC composite was prepared by hydrothermal method. The results indicated that the FeS2/MPC composite electrode exhibited better electrochemical performance than pristine FeS2. Especially, the discharge capacity of composite electrode reached 650 mAh g(-1) at 0.5 C current density, and this was significantly higher than that of pristine FeS2.

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