4.8 Article

Reversible polymer-gel transition for ultra-stretchable chip-integrated circuits through self-soldering and self-coating and self-healing

Journal

NATURE COMMUNICATIONS
Volume 12, Issue 1, Pages -

Publisher

NATURE PORTFOLIO
DOI: 10.1038/s41467-021-25008-5

Keywords

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Funding

  1. Carnegie Mellon-Portugal project WoW of the European Regional Development Fund (ERDF) [45913]
  2. Dermotronics - EU Structural & Investment Funds (FEEI) through an operational program of the center region [PTDC/EEIROB/31784/2017]
  3. Foundation of Science and Technology (FCT) of Portugal
  4. Add.Additive - Regional Development Funds (FEDER), through Programa Operacional Competitividade e InternacionalizacAo (POCI) [POCI-01-0247-FEDER-024533]
  5. QREN-Mais Centro program [ICT_2009_02_012_1890]

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The Pol-Gel technology enables low-cost, scalable, and rapid fabrication of hybrid microchip-integrated ultra-stretchable circuits through self-soldering, self-encapsulation, and self-healing, achieving maximum strain tolerance 5 times higher than previous works. This approach opens up new possibilities for applications of printed stretchable devices and soft circuits.
Integration of solid-state microchips into soft-matter, and stretchable printed electronics has been the biggest challenge against their scalable fabrication. We introduce, Pol-Gel, a simple technique for self-soldering, self-encapsulation, and self-healing, that allows low cost, scalable, and rapid fabrication of hybrid microchip-integrated ultra-stretchable circuits. After digitally printing the circuit, and placing the microchips, we trigger a Polymer-Gel transition in physically cross-linked block copolymers substrate, and silver liquid metal composite ink, by exposing the circuits to the solvent vapor. Once in the gel state, microchips penetrate to the ink and the substrate (Self-Soldering), and the ink penetrates to the substrate (Self-encapsulation). Maximum strain tolerance of similar to 1200% for printed stretchable traces, and >500% for chip-integrated soft circuits is achieved, which is 5x higher than the previous works. We demonstrate condensed soft-matter patches and e-textiles with integrated sensors, processors, and wireless communication, and repairing of a fully cut circuits through Pol-Gel.

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