Journal
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA
Volume 118, Issue 22, Pages -Publisher
NATL ACAD SCIENCES
DOI: 10.1073/pnas.2103696118
Keywords
time-resolved resonant X-ray scattering; transient magnetic excitations; iridates
Categories
Funding
- US Department of Energy (DOE) , Office of Science, Basic Energy Sciences, Materials Science and Engineering Division [DE-SC0012704, DEAC0206CH11357]
- Swiss National Science Foundation [P2EZP2_175092]
- Engineering and Physical Sciences Research Council (EPSRC) Centre for Doctoral Training in the Advanced Characterization of Materials [EP/L015277/1]
- ShanghaiTech University startup fund MOST of China [2016YFA0401000]
- National Natural Science Foundation of China [11934017]
- Chinese Academy of Sciences [112111KYSB20170059]
- EPSRC [EP/N027671/1, EP/N034872/1]
- Spanish Ministry of Economy and Competitiveness through the Severo Ochoa program for Centers of Excellence in RD [SEV20150522]
- Fundaci oPrivada Cellex
- Fundaci o MirPuig
- Generalitat de Catalunya through the CERCA program
- European Research Council under the European Union's Horizon 2020 research and innovation program [758461]
- NSF [DMR1848269]
- DOE Office of Science User Facility [DEAC0276SF00515]
- European Research Council (ERC) [758461] Funding Source: European Research Council (ERC)
- Swiss National Science Foundation (SNF) [P2EZP2_175092] Funding Source: Swiss National Science Foundation (SNF)
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Using ultrafast resonant inelastic X-ray scattering, we have shown that femtosecond laser pulses can excite transient magnons at large wavevectors in gapped antiferromagnets, persisting for several picoseconds. Our work suggests that materials with isotropic magnetic interactions are preferred for achieving rapid manipulation of magnetism.
Although ultrafast manipulation of magnetism holds great promise for new physical phenomena and applications, targeting specific states is held back by our limited understanding of how magnetic correlations evolve on ultrafast timescales. Using ultrafast resonant inelastic X-ray scattering we demonstrate that femtosecond laser pulses can excite transient magnons at large wavevectors in gapped antiferromagnets and that they persist for several picoseconds, which is opposite to what is observed in nearly gapless magnets. Our work suggests that materials with isotropic magnetic interactions are preferred to achieve rapid manipulation of magnetism.
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