4.8 Article

Spin-textured Chern bands in AB-stacked transition metal dichalcogenide bilayers

Publisher

NATL ACAD SCIENCES
DOI: 10.1073/pnas.2112673118

Keywords

moire superlattice; topological bands; first principle simulation; continuum model

Funding

  1. Department of Energy Office of Basic Energy Sciences, Division of Materials Sciences [DE-SC0018945, DE-SC0020149]
  2. Simons Foundation
  3. David and Lucile Packard Foundation
  4. U.S. Department of Energy (DOE) [DE-SC0018945, DE-SC0020149] Funding Source: U.S. Department of Energy (DOE)

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The study reveals the formation of topological moire bands induced by displacement fields in AB-stacked TMD heterobilayers and provides a method for creating such bands. This establishes a tunable platform for realizing quantum-spin Hall and interaction-induced quantum anomalous Hall effects.
While transition-metal dichalcogenide (TMD)-based moire ' materials have been shown to host various correlated electronic phenomena, topological states have not been experimentally observed until now [T. Li et al., Quantum anomalous Hall effect from intertwined moire bands. arXiv [Preprint] (2021). https://arxiv.org/abs/2107.01796 (Accessed 5 July 2021)]. In this work, using first-principle calculations and continuum modeling, we reveal the displacement field-induced topological moire bands in AB-stacked TMD heterobilayer MoTe2/WSe2. Valley-contrasting Chern bands with nontrivial spin texture are formed from interlayer hybridization between MoTe2 and WSe2 bands of nominally opposite spins. Our study establishes a recipe for creating topological bands in AB-stacked TMD bilayers in general, which provides a highly tunable platform for realizing quantum-spin Hall and interaction-induced quantum anomalous Hall effects.

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