Journal
MATERIALS TODAY
Volume 51, Issue -, Pages 449-474Publisher
ELSEVIER SCI LTD
DOI: 10.1016/j.mattod.2021.08.005
Keywords
Solid-state lithium metal batteries; Polymer electrolytes; Functional units adjustment; Interface stability; In-situ polymerization
Categories
Funding
- National Key R&D Program of China [2018YFB0104300]
- National Natu-ral Science Foundation of China [21875007, 22075007, 21975006, 51802009, 21974007]
- Beijing Natural Science Foundation [JQ19003, KZ202010005007, L182009]
- Pro-ject of Youth Talent Plan of Beijing Municipal Education Com-mission [CITTCD201804013]
- High-grade discipline construction of Beijing [PXM2019-014204-500031]
Ask authors/readers for more resources
This review discusses the development of polymer electrolytes through design strategies involving functional unit adjustments, as well as introducing the interfaces between polymer electrolytes and electrodes, interface issues, remedy strategies, and in-situ polymerization methods to enhance battery performance.
The polymer electrolyte based solid-state lithium metal batteries are the promising candidate for the high-energy electrochemical energy storage with high safety and stability. Moreover, the intrinsic properties of polymer electrolytes and interface contact between electrolyte and electrodes have played critical roles for determining the comprehensive performances of solid-state lithium metal batteries. In this review, the development of polymer electrolytes with the design strategies by functional units adjustments are firstly discussed. Then the interfaces between polymer electrolyte and cathode/anode, including the interface issues, remedy strategies for stabilizing the interface contact and reducing resistances, and the in-situ polymerization method for enhancing the compatibilities and assembling the batteries with favorable performances, have been introduced. Lastly, the perspectives on developing polymer electrolytes by functional units adjustment, and improving interface contact and stability by effective strategies for solid-state lithium metal batteries have been provided.
Authors
I am an author on this paper
Click your name to claim this paper and add it to your profile.
Reviews
Recommended
No Data Available