4.5 Article

Spin reorientation transition induced by surface reconstruction in epitaxial Fe/Co bilayers

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ELSEVIER
DOI: 10.1016/j.jmmm.2021.168019

Keywords

Spin reorientation transition; Magnetic anisotropy; Surface reconstruction; Magnetic interface anisotropy

Funding

  1. National Key Research and Development Program of China [2019YFB2005800]
  2. Natural Science Foundation of China [51625101, 51971026, 11874082]
  3. ISF-NSFC Joint Research Program [51961145305]
  4. Beijing Natural Science Foundation Key Program [Z190007]
  5. State Key Laboratory for Advanced Metals and Materials [2019Z-10]
  6. Fundamental Research Funds for the Central Universities [FRF-TP-16-001C2]

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Surface reconstruction influences the in-plane magnetic anisotropy of epitaxial Fe/Co bilayers, especially leading to a reconstruction-dependent in-plane spin reorientation transition at a Co layer thickness of 3 nm. This transition is attributed to the significantly enhanced magnetic interface anisotropy of Fe/Co bilayers due to the reconstruction.
Surface reconstruction is a common physical phenomenon, driving the atoms near the surface to form a different spacing or symmetry from the bulk atoms to minimize the free enthalpy of the system. The formation of an asymmetric (7 x 2) reconstruction was observed on (1 1 2)-oriented Fe surface, which may be related to the anisotropic strain distribution induced by lattice mismatch. The influence of reconstruction on in-plane magnetic anisotropy has been studied in epitaxial Fe/Co bilayers grown by molecular beam epitaxy. The evolutions of Co layer thickness-dependent magnetic anisotropy for reconstructed and unreconstructed configurations were investigated by magneto-optic Kerr effect technique. The most significant difference caused by reconstruction took place when tCo = 3 nm, showing a reconstruction-dependent in-plane spin reorientation transition with a rotation of 90, which can be attributed to the dramatically enhanced magnetic interface anisotropy of Fe/Co bilayers.

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