4.7 Article

Atmospheric transport and deposition of microplastics in a subtropical urban environment

Journal

JOURNAL OF HAZARDOUS MATERIALS
Volume 416, Issue -, Pages -

Publisher

ELSEVIER
DOI: 10.1016/j.jhazmat.2021.126168

Keywords

Microplastics; Atmospheric deposition; Abundance; Characteristics; Potential sources

Funding

  1. National Natural Science Foundation of China [42077364, 41703095]
  2. Natural Science Foundation of Guangdong Province, China [2021A1515011568]
  3. Science of Technology Program of Guangdong, China [2019A141405034]
  4. National Key Research and Development Program of China [2018YFD0900604]
  5. Guangdong Province Universities and Colleges Pearl River Scholar Funded Scheme
  6. Key Research Projects of Universities in Guangdong Province [2019KZDXM003, 2020KZDZX1040]

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Microplastics pollution is a major environmental challenge, and the atmosphere plays a significant role in the global cycle of microplastics. This study analyzed atmospheric deposition of microplastics in urban Guangzhou, China, finding that fibers were the most abundant type and likely originated from textiles. Meteorological factors like rainfall and wind events were suggested to influence the transport and deposition of airborne microplastics.
As an issue of great concern, microplastics pollution has emerged as a key environmental challenge of our time. The atmosphere is a significant compartment in the global cycle of microplastics, however, studies on the transport and deposition of airborne microplastics is limited. In the present work, atmospheric wet and dry deposition of microplastics were analyzed over one year in an urban environment of megacity Guangzhou, China. The atmospheric deposition fluxes of microplastics ranged from 51 to 178 particles/m2/d (mean: 114 +/- 40 particles/m2/d). Fibers, fragments, films and microbeads were observed in the deposition samples, with fibers being the most abundant microplastics, accounting for 77.6 +/- 19.1% of the total. The chemical composition of microplastics were identified using micro Fourier transform infrared spectrometer. 78.7% of the fibrous microplastics were derived from petrochemicals and most were polyethylene terephthalate (polyester), suggesting that textiles (e.g., clothes and curtains) were likely the main source. The results of back-trajectory analysis indicated that city rivers may act as secondary sources of airborne microplastics. Though no significant correlation was found between atmospheric microplastic deposition and meteorological factors such as rainfall and wind events, these factors were suggested to be positive drivers for the transport and deposition of airborne microplastic.

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