4.7 Article

Green recycling of fly ash into heat and sound insulation composite aerogels reinforced by recycled polyethylene terephthalate fibers

Journal

JOURNAL OF CLEANER PRODUCTION
Volume 322, Issue -, Pages -

Publisher

ELSEVIER SCI LTD
DOI: 10.1016/j.jclepro.2021.129138

Keywords

Fly ash; Recycled polyethylene terephthalate; Composite aerogel; Heat insulation; Sound insulation

Funding

  1. Ho Chi Minh City Foundation for Science and Technology Development [120/2019/HDQPTKHCN]

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By converting fly ash into a lightweight composite aerogel reinforced with recycled polyethylene terephthalate fiber, a feasible zero-waste method has been developed to address environmental pollution, resulting in aerogels with extremely low density, high porosity, low thermal conductivity, flexibility, and noise reduction. This study offers a safe, environmentally friendly, and cost-effective solution for recycling fly ash into high-value engineering materials.
Fly ash is waste from thermal power plants that not only has a serious impact on soil and water but also accumulates in landfills and must be treated properly. In addition, plastic waste, especially polyethylene terephthalate bottles, deteriorates for a long time, so there is an urgent need to recycle them into valuable products. To solve the environmental pollution mentioned above, a feasible zero-waste method has been developed that converts 100% of fly ash into a lightweight composite aerogel reinforced with recycled polyethylene terephthalate fiber. In this study, raw fly ash is bound to the skeleton of the fibers by a non-toxic, biodegradable xanthan gum solution as a binder, which is then lyophilized, leaving a hollow porous structure. The obtained composite aerogels display extremely low density of 0.026-0.062 g/cm(3), high porosity of 96.59-98.42%, low thermal conductivity of 34-39 mW/(m.K), flexibility with Young's modulus of 3.98-20.61 kPa, and noise reduction coefficient of 0.18-0.31. Adding fly ash to the fiber framework results in a lightweight composite aerogel with higher porosity, heat, and acoustic insulation, as well as impressive compressive modulus, compared to the fly ash-free aerogels. This study provides a safe, environmentally friendly, and cost-effective solution for recycling fly ash into high-value engineering materials.

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