4.7 Article

Dynamic behavior of droplet transport on realistic gas diffusion layer with inertial effect via a unified lattice Boltzmann method

Journal

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
Volume 46, Issue 66, Pages 33260-33271

Publisher

PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.ijhydene.2021.07.124

Keywords

Lattice Boltzmann method; Fuel cells; Gas diffusion layer; 3D flow channels; Liquid droplet transport

Funding

  1. National Key R&D Program of China [2020YFB0106604]
  2. UK Consortium on Mesoscale Engineering Sciences (UKCOMES) under the UK Engineering and Physical Sciences Research Council [EP/R029598/1]
  3. EPSRC [EP/R029598/1] Funding Source: UKRI

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The study investigates the dynamic behavior of liquid droplets on a reconstructed real gas diffusion layer (GDL) surface with inertial effects from a 3D flow channel using an improved pseudopotential multiphase model within the ULBM framework. Results show that the droplet behavior on the surface is influenced by inertia and contact angles.
The dynamic behavior of liquid droplets on a reconstructed real gas diffusion layer (GDL) surface with the inertial effect produced by the three dimensional (3D) flow channel is investigated using an improved pseudopotential multiphase model within the unified lattice Boltzmann model (ULBM) framework, which can realize thermodynamic consistency and tunable surface tension. The microstructure of the GDL (Toray-090) including carbon fibers and polytetrafluoroethylene (PTFE) is reconstructed by a stochastic and mixed-wettability model. The critical force formulation for the Cassie-Wenzel transition of a droplet on GDL surface is derived. The effects of inertia and contact angles on the liquid droplet transport process on a reconstructed real GDL surface with a 3D flow channel are investigated. The results show the normalized center-of-mass coordinate X may enter the channel wall area or fluctuate around the initial position. With increased inertia applied on the droplet, the normalized center-of-mass coordinate Y grows faster and the normalized center-of-mass coordinate Z decreases. It is found by the ULBM for the first time that the liquid droplet is pushed back into the GDL by inertial effect. With the increase of inertia and the decrease of contact angle of GDL, both the droplet penetration depth in GDL and the droplet invasion fraction increase. The droplet invasion fraction in GDL is up to 30%. (c) 2021 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.

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