Journal
ELECTROANALYSIS
Volume 34, Issue 2, Pages 362-368Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/elan.202100214
Keywords
Nanocomposite hydrogel; Gold nanoparticles; Pressure responsive; Electrochemiluminescence
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Funding
- National Natural Science Foundation of China [21575027]
- University of Fujian Province [2018Y4007]
- Natural Sciences Foundation of Fujian Province [2020J01968, 2020J05250]
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The functional nanocomposite hydrogel, utilizing distinctive porous matrix, luminophore, and functional nanoparticles, shows external pressure responsive properties and remarkable amplification of electrochemiluminescence signals. Furthermore, the uniform dispersion of luminophore over nanocomposite hydrogel significantly enhances the long term stability of ECL compared to conventional methods.
Synergistically taking the advantage of distinctive porous matrix, luminophore and functional nanoparticles, we prepared functional nanocomposite hydrogel combining the hydrophilic three-dimensional network of hydrogels as matrix for the adsorption of luminophore, Ru(bpy)(3)(2+), and in situ grown gold nanoparticles (AuNPs) as the conductive. Interestingly, the designed nanocomposite hydrogel shows external pressure resposnsive properties, which precisely tune the distance between the AuNPs becomes shorter, resulting in a remarkable amplification of electrochemiluminescence (ECL) signals. Additionally, differing from the poor stability of conventional ECL, uniform dispersion of the Ru(bpy)(3)(2+) over nanocomposite hydrogel significantly enhanced the long term stability of ECL.
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