Journal
FARADAY DISCUSSIONS
Volume 194, Issue -, Pages 305-324Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c6fd00103c
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Funding
- Max Planck Society
- Knut and Alice Wallenberg Foundation [KAW-2013.0020]
- Swedish Research Council (VR)
- Science and Technology Facilities Council (STFC)
- U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical, Geological, and Biological Sciences [DE-AC02-06CH11357]
- U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-76SF00515]
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With the invention of femtosecond X-ray free-electron lasers (XFELs), studies of light-induced chemical reaction dynamics and structural dynamics reach a new era, allowing for time-resolved X-ray diffraction and spectroscopy. To ultimately probe coherent electron and nuclear dynamics on their natural time and length scales, coherent nonlinear X-ray spectroscopy schemes have been proposed. In this contribution, we want to critically assess the experimental realisation of nonlinear X-ray spectroscopy at current-day XFEL sources, by presenting first experimental attempts to demonstrate stimulated resonant X-ray Raman scattering in molecular gas targets.
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