Journal
CHEMISTRY-AN ASIAN JOURNAL
Volume 16, Issue 21, Pages 3487-3491Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/asia.202100833
Keywords
alpha-amino tertiary alkylperoxides; 1,3,5-triazines; peroxidation; Lewis acid
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Funding
- Shenzhen Development and Reform Committee [2019156]
- Shenzhen Science, Technology and Innovation Commission [JCYJ20180306174248782]
- Department of Science and Technology of Guangdong Province [2017B030314083]
- Shenzhen Bay Laboratory Open Funding [SZBL2019062801009]
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This study has developed a novel reaction method for the efficient synthesis of diverse α-amino tertiary alkylperoxides. Mechanistic investigations and useful synthetic applications of the products have also been presented.
alpha-Substituted peroxides have been found in natural products and are widely used as anti-malarial agents. Zn(OTf)(2)-catalyzed peroxidation of 1,3,5-triazines has been developed, accessing diversely substituted alpha-amino tertiary alkylperoxides with high efficiency. Mechanistic investigations and useful synthetic application of the products have also been presented.
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