Journal
BIORESOURCE TECHNOLOGY
Volume 329, Issue -, Pages -Publisher
ELSEVIER SCI LTD
DOI: 10.1016/j.biortech.2021.124876
Keywords
KELM; Kriging; Biochar; Stepwise regression analysis; Sensitivity analysis
Funding
- National Natural Science Foundation of China [41807196]
- Postdoctoral Science Foundation of Heilongjiang Province of China [LBHZ19002]
- Open Research Fund of State Key Laboratory of Geomechanics and Geotechnical Engineering, Institute of Rock and Soil Mechanics, Chinese Academy of Sciences [Z019005]
- University Nursing Program for Young Scholars with Creative Talents in Heilongjiang Province [UNPYSCT2017018]
- Natural Science Foundation of Heilongjiang Province of China [QC2018019]
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The study introduces the use of KELM and Kriging models to predict the heavy metal adsorption efficiency of biochar, improving model fitting accuracy and identifying the strong relationship between adsorption efficiency and pHsolute and T. The most sensitive parameters are T, pHH2O, r, C, and pHsolute. Accurate predictive models help reduce the number of experiments needed for metal-biochar adsorption in the future.
Kernel extreme learning machine (KELM) and Kriging models are proposed to predict biochar adsorption efficiency of heavy metals. Both six popular ions (Pb2+, Cd2+, Zn2+, Cu2+, Ni2+, As3+) and single ion are considered to test the accuracy of KELM and Kriging models. Two ways (data selection and fix output value) are attempted to improve the model fitting accuracy and the best R2 can reach 0.919 (KELM) and 0.980 (Kriging). In addition, stepwise regression and local sensitivity analysis show that adsorption efficiency has strong relationship with pHsolute and T. Moreover, the most sensitive parameters are T, pHH2O, r, C and pHsolute. The accurate KELM and Kriging models identify the most important controlling factors on metal adsorption, and ultimately provide some sort of predictive framework that will be useful in selecting appropriate biochar for particular treatment scenarios. This, in turn, will reduce the number of metal-biochar adsorption experiments needed going forward.
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