Journal
AICHE JOURNAL
Volume 67, Issue 9, Pages -Publisher
WILEY
DOI: 10.1002/aic.17337
Keywords
fludization; mathematical modeling; multi-phase flow; multiscale modeling; particle technology
Categories
Funding
- Dow Chemical Company
- National Science Foundation [ACI-1532236, ACI-1532235]
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The study suggests that a force-based description is more suitable for enduring-contact systems, while an energy-based description is more suitable for brief-contact systems in cohesive-particle interactions. By collapsing dimensionless variables against two dimensionless numbers, the hypothesis is supported by experimental and simulation systems, providing new insights into Geldart's classification.
Much confusion exists on whether force- or energy-based descriptions of cohesive-particle interactions are more appropriate. We hypothesize a force-based description is appropriate when enduring-contacts dominate and an energy-based description when contacts are brief in nature. Specifically, momentum is transferred through force-chains when enduring-contacts dominate and particles need to overcome a cohesive force to induce relative motion, whereas particles experiencing brief contacts transfer momentum through collisions and must overcome cohesion-enhanced energy losses to avoid agglomeration. This hypothesis is tested via an attempt to collapse the dimensionless, dependent variable characterizing a given system against two dimensionless numbers: A generalized bond number, Bo(G)-ratio of maximum cohesive force to the force driving flow, and a new Agglomerate number, Ag-ratio of critical cohesive energy to the granular energy. A gamut of experimental and simulation systems (fluidized bed, hopper, etc.), and cohesion sources (van der Waals, humidity, etc.), are considered. For enduring-contact systems, collapse occurs with Bo(G) but not Ag, and vice versa for brief-contact systems, thereby providing support for the hypothesis. An apparent discrepancy with past work is resolved, and new insight into Geldart's classification is gleaned.
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