4.8 Article

MoTe2: Semiconductor or Semimetal?

Journal

ACS NANO
Volume 15, Issue 8, Pages 12465-12474

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acsnano.1c01816

Keywords

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Funding

  1. National Research Foundation Singapore [NRF-CRP22-2019-0007, NRF-CRP21-2018-0007]
  2. Ministry of Education, Singapore, under its AcRF Tier 3 Programme Geometrical Quantum Materials [MOE2018-T3-1-002]
  3. Singapore NTU Presidential Postdoctoral Fellowship [03INS000973C150]
  4. National Basic Research Program of China from the MOST [2016YFA0300601, 2014CB920904, 2015CB921402]
  5. National Natural Science Foundation of China [92065203, 11527806, 11874406]
  6. Beijing Municipal Science & Technology Commission of China [Z191100007219008]
  7. Beijing Academy of Quantum Information Sciences [Y18G08]
  8. Strategic Priority Research Program of the Chinese Academy of Sciences [XDB33010300]
  9. Synergic Extreme Condition User Facility

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Transition metal tellurides (TMTs) have attracted intense interest due to their diverse phase topologies, exhibiting a wide range of physical properties such as acting as topological insulators, semiconductors, Weyl semimetals, and superconductors. Among the TMT families, MoTe2 stands out as a representative material with its Janus nature and rich phases. This Perspective introduces the phase structures and synthesis strategies of MoTe2, focusing on recent advances and emerging quantum states of Janus MoTe2, along with insights into the opportunities and challenges in device design and applications associated with MoTe2.
Transition metal tellurides (TMTs) have attracted intense interest due to their intriguing physical properties arising from their diverse phase topologies. To date, a wide range of physical properties have been discovered for TMTs, including that they can act as topological insulators, semiconductors, Weyl semimetals, and superconductors. Among the TMT families, MoTe2 is a representative material because of its Janus nature and rich phases. In this Perspective, we first introduce phase structures in monolayer and bulk MoTe2 and then summarize MoTe2 synthesis strategies. We highlight recent advances of Janus MoTe2 in terms of material structures and emerging quantum states. We also provide insight into the opportunities and challenges faced by MoTe2-associated device design and applications.

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