Journal
ACS APPLIED ENERGY MATERIALS
Volume 4, Issue 4, Pages 3101-3109Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acsaem.0c02831
Keywords
LiNi0.5Mn1.5O4; Li-ion microbatteries; thin lms; sputtered films; surface capacities; faradic process
Funding
- CASSIOPES project [ANR-17-CE09-0016-01]
- French network on electrochemical energy storage (RS2E)
- STORE-EX Labex
- Chevreul Institute [FR 2638]
- Ministere de l'Enseignement Superieur et de la Recherche
- Region Hauts de France
- FEDER
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This paper presents a detailed study on the influence of sputtering deposition parameters on the electrochemical properties of electrodes for lithium-ion microbatteries. The research aims to optimize the performance and investigate the relationship between structure and electrochemical properties.
To power miniaturized and smart electronic devices, lithium-ion microbatteries with high energy densities remain the most attractive solution. The Ni-substituted LiMn2O4, spinet material seems to be the most promising high-performance electrodes to significantly enhance the energy density of Li-ion microbatteries. Sputtered LiNi0.5Mn1.5O4 (LNMO) films deposited on a metallic current collector are known to deliver high capacity values with high rate capabilities. In this paper, we propose a detailed study on the influence of sputtering deposition parameters (gas flow rate and bias voltage) to optimize the electrochemical properties of the electrodes and to carefully investigate the structure-electrochemical property relationship.
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