Journal
MATERIALS TODAY ENERGY
Volume 21, Issue -, Pages -Publisher
ELSEVIER SCI LTD
DOI: 10.1016/j.mtener.2021.100781
Keywords
UIO-66 membrane; Nano-SAPO-34; Pt NPs; Core-shell catalysts; CO2 hydrogenation
Funding
- National Natural Science Foundation of China [U1862204, 21878090, 21371058]
- National Natural Science Foundation of PetroChina [U1862204]
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By modifying the SAPO-34 catalyst with UIO-66 membrane, the carbon monoxide yield and CO selectivity have been improved. This demonstrates an enhancement in carbon dioxide conversion efficiency.
The core-shell catalyst Pt/SAPO-34@UIO-66, Haibao-like cluster, was prepared. The Haibao-like cluster was from Zr-based metal-organic framework UIO-66 coating and grows epitaxially on the surface of nano-SAPO-34 clusters and Pt nanoparticles uniformly dispersed on the UIO-66 membrane. The catalyst Pt/SAPO-34@UIO-66 increases carbon monoxide yield compared with catalysts Pt/SAPO-34 and Pt/UIO-66, and the synergy effect of UIO-66 membrane improves carbon monoxide(CO) selectivity. This proves that the modification of SAPO-34 with UIO-66 membrane can enhance the carbon dioxide conversion efficiency. (C) 2021 Elsevier Ltd. All rights reserved.
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