4.6 Article

Flexible Self-Charging, Ultrafast, High-Power-Density Ceramic Capacitor System

Journal

ACS ENERGY LETTERS
Volume 6, Issue 4, Pages 1383-1391

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acsenergylett.1c00170

Keywords

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Funding

  1. NRF - Korea government (MSIT) [2019R1C1C1003765, 2019R1A2B5B01070100]
  2. National Research Council of Science & Technology (NST) grant by the Korea government (MSIP) [CAP-1704-KRISS]
  3. Convergent Technology R&D Program for Human 1893 Augmentation through the National Research Foundation of Korea [NRF-2020M3C1B8081519]
  4. National Research Foundation of Korea (NRF) - Korea government (MSIT) [2020R1F1A1051206]
  5. National Research Foundation of Korea [2020R1F1A1051206, 2020M3C1B8081519, 2019R1A2B5B01070100, 2019R1C1C1003765] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)

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The flexible self-charging, ultrafast, and high-power-density (SUHP) capacitor system demonstrated in this study integrates an aerosol-deposited nanograined relaxor ferroelectric Pb(Mg1/3Nb2/3)O-3-PbTiO3 (PMN-PT) capacitor and piezoelectric Pb(Zr-x,Ti1-x)O-3 (PZT) harvester, generating electric energy under biomechanical bending force and storing it for discharge with high energy density and power density, showcasing a promising approach for powering future flexible pulsed-power electronic devices.
Flexible self-charging capacitor systems, which exhibit the combined functions of energy generation and storage, are considered a promising solution for powering flexible self-powered electronics. Here, we present a new approach to demonstrate a flexible self-charging, ultrafast, and high-power-density (SUHP) capacitor system by integrating an aerosol-deposited nanograined relaxor ferroelectric Pb(Mg1/3Nb2/3)O-3-PbTiO3 (PMN-PT) capacitor and piezoelectric Pb(Zr-x,Ti1-x)O-3 (PZT) harvester. The as-designed flexible SUHP capacitor system can generate electric energy with an open-circuit voltage of 172 V and a short-circuit current of 21 mu A under a biomechanical bending force of human fingers. This energy can be stored in the integrated flexible capacitor part and then discharged with a high energy density of 2.58 J/cm(3) within an ultrafast time of 480 ns. Moreover, a high power density of 5.38 MW/cm(3) from the flexible SUHP capacitor suggests that the proposed approach for self-charging and energy storage may be an efficacious way to drive future flexible pulsed-power electronic devices.

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