4.7 Article

X-ray Photoemission Spectroscopy Study of Uniaxial Magnetic Anisotropy Induced in a Ni Layer Deposited on a LiNbO3 Substrate

Journal

NANOMATERIALS
Volume 11, Issue 4, Pages -

Publisher

MDPI
DOI: 10.3390/nano11041024

Keywords

heterojunction; magnetic anisotropy; magnetoelastic effect; X-ray photoemission spectroscopy; X-ray magnetic circular dichroism photoemission electron microscopy

Funding

  1. JSPS [17H02755]
  2. Shimadzu science and technology foundation
  3. Japan Synchrotron Radiation Research Institute (JASRI) [2018A1317, 2019A1404, 2019B1345]
  4. Grants-in-Aid for Scientific Research [17H02755] Funding Source: KAKEN

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The research focuses on the competition between magnetic shape anisotropy and induced uniaxial magnetic anisotropy in the heterojunction between a ferromagnetic layer and a ferroelectric substrate. It reveals the origin of the uniaxial magnetic anisotropy induced from the heterojunction and provides a means for simultaneous control of magnetism, mechanics, and electronics in nano/microsystems consisting of ferromagnetic/ferroelectric materials.
The competition between magnetic shape anisotropy and the induced uniaxial magnetic anisotropy in the heterojunction between a ferromagnetic layer and a ferroelectric substrate serves to control magnetic domain structures as well as magnetization reversal characteristics. The uniaxial magnetic anisotropy, originating from the symmetry breaking effect in the heterojunction, plays a significant role in modifying the characteristics of magnetization dynamics. Magnetoelastic phenomena are known to generate uniaxial magnetic anisotropy; however, the interfacial electronic states that may contribute to the uniaxial magnetic anisotropy have not yet been adequately investigated. Here, we report experimental evidence concerning the binding energy change in the ferromagnetic layer/ferroelectric substrate heterojunction using X-ray photoemission spectroscopy. The binding energy shifts, corresponding to the chemical shifts, reveal the binding states near the interface. Our results shed light on the origin of the uniaxial magnetic anisotropy induced from the heterojunction. This knowledge can provide a means for the simultaneous control of magnetism, mechanics, and electronics in a nano/microsystem consisting of ferromagnetic/ferroelectric materials.

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